Preferred Language
Articles
/
jih-4332
New Phenolic-Carbonyl Azo Ligand and its Binding Modes, Geometry Assignments and Thermal Behavior for Ligand and its Metal Complexes
...Show More Authors

A fabricated Azo ligand (E)-1-[4-(3,4-dichloro-2-hydroxyphenyl) diazenyl] phenylethan-1-one was produced by a coupling reaction between diazonium salt made from p-aminoacetophenone and a basic solution of 2,3-dichlorophenol. The azo compound was used to form complexes with Cr(III), Co(II), Ni(II), and Cu(II) ions at a 2L:1M molar ratio in an alcoholic medium. The ligand and its complexes were characterized using a set of spectroscopic techniques to obtain chemical and structural information. Infrared with Fourier transformation; ultraviolet and visible; ¹H/¹³C nuclear magnetic resonance; mass; thermal analysis and micro elemental analysis spectrometry, as well as molar conductivity. The results certified the chemical moiety and geometric fabrication. Azo dye acts as a bidentate ligand with phenol/hydroxy terminals. The finding was that Cr(III), Co(II), and Ni(II) complexes were characterized by a six-coordinate (distorted octahedral) geometry, whereas the Cu(II) complex had a tetrahedral structure. Thermal decomposition of the ligand and the selected complex was studied to assess stability upon heating and to determine the final residue.

View Publication Preview PDF
Quick Preview PDF